How to Say "surly" in Spanish
The Spanish word for “surly” is “agrio” — B2 level.
English → SpanishB2
adjectiveB2
unfriendly behavior

Examples
Desde que perdió su trabajo, tiene un carácter muy agrio.
Since he lost his job, he has a very bitter personality.
Me dio una respuesta agria cuando le pedí ayuda.
She gave me a harsh response when I asked for help.
Metaphorical Use
Just like in English, words for taste are used to describe personalities. A 'sour' person is someone who is unfriendly or grumpy.
Don't use for 'sad'
Mistake: “Estoy agrio porque mi gato murió.”
Correction: Estoy triste porque mi gato murió.
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